Beryllium chemical combination has a considerable effect on the design and fabrication of the 241 Am -9 Be neutron source. In this investigation the beryllium combinations were studied as a generator of neutrons with various mass percentage, and the neutron yields were also calculated using the results of the ALICE and SRIM codes calculations per unit incident charge. The neutron yields of Beryllium Hydride, Beryllium Carbide, Beryllium Hydroxide, Beryllium Oxide, Beryllium Acetate, Beryllium Acetylacetonate and Beryllium Sulfate were calculated as 4397.992 ´ 10-7, 1511.184 ´ 10-7, 976.609 ´ 10-7, 595.299 ´ 10-7, 336.163 ´ 10-7, 169.62 ´ 10-7and 149.053 ´ 10-7respectively. Our calculations indicate that, the Beryllium Hydride is a proper material for use in the241 Am -9 Be neutron source.